The constitutional court banned the vote and almost 900 people were hurt as police tried to stop it going ahead.
More than 2.2 million people were reported to have voted, according to Catalan authorities, out of 5.3 million registered voters. Just under 90% of those who voted backed independence, they said.
In Girona, riot police smashed their way into a polling station where Mr Puigdemont was due to vote, and forcibly removed those inside. He voted at another station.
Large crowds of independence supporters gathered in the centre of the regional capital Barcelona on Sunday evening, waving flags and singing the Catalan anthem. Anti-independence protesters have also held rallies in Barcelona and other Spanish cities.
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